Proceedings of nanoGe Spring Meeting 2022 (NSM22)
DOI: https://doi.org/10.29363/nanoge.nsm.2022.143
Publication date: 7th February 2022
Metal halide perovskite solar cells have gained tremendous attention due to their high power conversion efficiencies and potential for low‐cost manufacturing. Their wide and tunable bandgap makes perovskites ideal candidates for tandem solar cells with narrow bandgap photovoltaic technologies, such as crystalline silicon, Cu(In,Ga)Se2, and low-bandgap perovskite, to go beyond the efficiency beyond the Shockley–Queisser single-junction limit. The past 5 years have witnessed unprecedented advancements in perovskite-based tandems, with lab-scale devices (up to around 1cm2) approaching or even surpassing efficiency records of their single-junction building blocks. Currently, the majority of the perovskite-based tandems are fabricated on rigid glass substrates. It is highly desirable to develop perovskite tandem solar cells on flexible and lightweight substrates. This would open up the possibilities for high throughput roll-to-roll manufacturing and various attractive applications including the portable and wearable electronics, smart buildings, transportations, etc., where a combination of high efficiency, lightweight, and flexibility are important considerations. In this contribution, we will present our progress on developing highly efficient flexible wide-bandgap perovskite solar cells with high near-infrared transmittance and flexible narrow-bandgap CIGS and Pb-Sn perovskite solar cells. We demonstrate over 22% and 24% in all-perovskite and perovskite-CIGS flexible thin film tandems, respectively.