Proceedings of Materials for Sustainable Development Conference (MAT-SUS) (NFM22)
DOI: https://doi.org/10.29363/nanoge.nfm.2022.214
Publication date: 11th July 2022
Organic-inorganic hybrid perovskite photovoltaics have attracted tremendous attention due to rapid progress in terms of power conversion efficiency in the last few years, from 3.8% to present record values in excess of 25%. However, fundamental problems, such as the toxicity of hybrid lead halide perovskites, hysteresis and structural instability remain to be solved for their application and commercialization. Indeed, the low-temperature solution-processing of perovskite films inevitably causes formation of a certain amount of defects on the surface and at the grain boundaries, which lead to serious trapping, charge accumulation, and recombination problems as well as stability issue. We pursue the interface engineering, defects passivation, and dimensional tunability approaches via introducing various types of multifunctional conjugated organic compounds to improve the stability and performance of perovskite photovoltaics.
In this presentation, we will discuss our achieved results in details for the above-mentioned approaches with a central focus on the fundamental complexity of microstructure and charge transport mechanisms and their correlation to the device performance, stability and indoor application.