Enabling accelerated PV materials and device development and deployment
Eva Unger a b
a Helmholtz Zentrum Berlin für Materialien und Energie,, Hahn-Meitner-Platz, 1, Berlin, Germany
b Department of Chemistry and NanoLund, Lund, Suecia, Lund, Sweden
Materials for Sustainable Development Conference (MATSUS)
Proceedings of Materials for Sustainable Development Conference (MAT-SUS) (NFM22)
#OPTONEXT - Next Gen Semiconductors for Optoelectronics
Barcelona, Spain, 2022 October 24th - 28th
Organizers: Paul Shaw and Mike Hambsch
Invited Speaker, Eva Unger, presentation 207
DOI: https://doi.org/10.29363/nanoge.nfm.2022.207
Publication date: 11th July 2022

To enable sustainable and low-cost energy conversion technology – the development of new energy conversion technology needs to be accelerated. In this talk, our approach to make use of scalable manufacturing methods to accelerate the optimization of process of functional materials research by combinatorial synthesis is described. We have been able to demonstrate to solution-based scalable combinatorial methods based on slot-die coating and inkjet printing [1,2]. We have managed to synthesize homogeneous combinatorially inkjet-printed samples of halide perovskite semiconductors [1,2] and evaluate the phase diagram and compositional homogeneities of these samples. Becoming involved in combinatorial science, we have also become very active and involved to set up materials databases and create tools enabling faster technology development in line with FAIRdata principles. We mobilized >90 scientist from our research community to help accumulate the information distributed over 17000 publication on the fabrication and resulting performance metrics in halide perovskite solar cells.[3] The resulting database - The Perovskite Database - with integrated interactive graphical tools for data visualization and searching hase been released (www.perovskitedatabase.com) and can now be made use for experimental data dissemination by the world-wide perovskite PV community. Another factor in accelerating materials development is the utilization and development of in-line process analytics, which enables us to gain direct feedback during materials processing to help find optimal process conditions and ink compositions faster. Futhermore, we have developed a high-throughput materials discovery platform based on slot-die coating (http://just.science/in-form/), which will enable high-throughput X-ray based synchrotron experimentation at the Balder beamline at MAXIV. A last but very important step is also the fabrication of larger area prototypes to enable the evaluation of new materials on a higher technology readiness level and the validation in real operating conditions. Based on slot-die coating, we have been able to manufacturing perovskite PV minimodules with >20% power conversion efficiencies, that we have also been able to encapsulate and try in an outdoor rooftop test station in Berlin. In all of our research activities we aim for early involvement of industrial partners to ensure direct pathways for technlogy transfer of our R&D.

We acknowledge funding from the German Ministry of Education and Research (BMBF) for the Young Investigator Group Hybrid Materials Formation and Scaling (HyPerFORME) within the program “NanoMatFutur” (grant no. 03XP0091) and the “SNaPSHoTs” project (grant no. 01IO1806). J.L. acknowledges funding from the Chinese Scholarship Council (CSC, grant no. CSC201908120116). E.U. and J.J. acknowledge funding from the Swedish Foundation for Strategic Research (SSF, Project ITM17-0276).The authors would like to acknowledge the use of the beam time at BESSYII, KMC-2 in Berlin and MAXIV in Sweden.

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