Helicity-dependent terahertz radiation of topological insulator Sb2Te3 nano thin film
Chien-Ming Tu a, Chih-Wei Luo b, Ping Huang b, Yi-Cheng Chen b, Pei-Yu Chuang c, Jung-Chun A Huang c, Ming-Yu Lin c, Jiunn-Yuan Lin d, Cheng-Maw Cheng e, Way-Faung Pong f, Takayoshi Kobayashi g
a Department of Physics, Lund University, P.O. Box 118, Lund, SE-221 00, Sweden
b National Chiao Tung University Hsinchu, Taiwan, 1001 University Road, Hsinchu, Hsinchu, Taiwan, Republic of China
c Department of Physics, National Cheng Kung University, No.1, University Road, Tainan City, 701, Taiwan, Republic of China
d National Chiao Tung University Hsinchu, Taiwan, 1001 University Road, Hsinchu, Hsinchu, Taiwan, Republic of China
e National Synchrotron Radiation Research Center, 101, Hsin-Ann road, Hsinchu Science Park, Hsinchu, 30076, Taiwan, Republic of China
f Department of Physics, Tamkang University, No.151, Yingzhuan Rd., Tamsui Dist., New Taipei City, 25137, Taiwan, Republic of China
g Advanced Ultrafast Laser Research Center, Department of Engineering Science, The University of Electro-Communications, -5-1 Chofugaoka, Chofu, Tokyo 182-8585, Japan
Materials for Sustainable Development Conference (MATSUS)Proceedings of September Meeting 2016 (NFM16)
Berlin, Germany, 2016 September 5th - 13th
Organizers: Marin Alexe, Enrique Cánovas, Celso de Mello Donega, Ivan Infante, Thomas Kirchartz, Maksym Kovalenko, Federico Rosei, Lukas Schmidt-Mende, Laurens Siebbeles, Peter Strasser, Teodor K Todorov, Roel van de Krol and Ulrike Woggon
Oral, Takayoshi Kobayashi, presentation 417
Publication date: 14th June 2016
Topological insulators (TIs) represent a new quantum phase of matter with a Dirac cone-like conducting surface state that shows time-reversal protection from backscattering due to spin-momentum-locking.Recently, some studies demonstrate that helicity-dependent photocurrent on TIs can be manipulated by the polarization of incident light. Reversing the helicity of circular polarized light reverses the direction of the helicity-dependent photocurrent. These works highlight the potential of TIs on applications of spintronics in the future.Here we demonstrate the terahertz (THz) emission spectroscopy of Sb2Te3 nano thin film under the excitation of ultrafast optical pulses of different helicity. In the oblique optical incidences, the polarity-reversals of the emitted THz waveform were observed as the polarization of optical pulse was changed from right-hand-circular-polarization to left-hand-circular-polarization. The helicity of optical pulses changes from +1 to -1 as well. In normal optical incident, no polarity-reversal of THz waveform was observed. A model based on transient photocurrent and optical rectification describes the experimental results very well. Comparing with the recent results on photocurrent measurements, we believe the phenomena are strongly related to the spin-polarized current on the surface of TIs.
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