Polaritonic Metasurface Based on Halide Perovskite
Nguyen Ha My Dang a, Simone Zanotti c, Celine Chevalier a, Gaëlle Trippé-Allard d, Emmanuel Drouard a, Dario Gerace c, Emmanuelle Deleporte d, Christian Seassal a, Hai Son Nguyen a b
a Univ Lyon, Ecole Centrale de Lyon, INSA Lyon, Université Claude Bernard Lyon 1, CPE Lyon, CNRS, INL, UMR5270, Ecully 69130, France
b Institut Universitaire de France - IUF
c Dipartimento di Fisica, Università di Pavia, via Bassi 6, I-27100 Pavia, Italy
d Lumière, Matière et Interfaces (LuMIn) Laboratory, Université Paris-Saclay, ENS Paris-Saclay, CNRS, CentraleSupélec, 91190 Gif-sur-Yvette, France
Materials for Sustainable Development Conference (MATSUS)
Proceedings of MATSUS Spring 2025 Conference (MATSUSSpring25)
Illuminating the Future: Advancements in Photon sources, Photodetectors, and Photonic Applications with 3D and low- dimensional metal halide perovskites - #PhotoPero
Sevilla, Spain, 2025 March 3rd - 7th
Organizers: Emmanuelle Deleporte, Blas Garrido and Juan P. Martínez Pastor
Invited Speaker, Hai Son Nguyen, presentation 419
DOI: https://doi.org/10.29363/nanoge.matsusspring.2025.419
Publication date: 16th December 2024

Exciton-polaritons are half-light, half-matter excitations arising from the strong coupling regime between cavity photons and excitons of semiconductors [1]. Behaving as superlative non-linear photons due to their hybrid nature, exciton-polaritons have been providing a fruitful ground for studying quantum fluid of light and realizing prospective all-optical devices. In this presentation, we present experimental studies on exciton-polaritons in resonant metasurfaces, which are composed of sub-wavelength lattices of perovskite pillars (see Figure). Room temperature polaritons are demonstrated with a remarkable Rabi splitting in the 200 meV range. We show that polaritonic dispersion can be tailored on-demand. This includes creating linear, slow-light,  multi-valley shaped dispersions [2] as well as polarization vortex emission [3]. Finally, we observe experimentally the ballistic propagation of polaritons over hundreds of micrometers at room temperature, even with large excitonic components, some up to 80%. This long-range propagation is enabled by the high homogeneity of the metasurface, and by the large Rabi splitting which completely decouples polaritons from the phonon bath at the excitonic energy [4]. Our results suggest a new approach to study exciton-polaritons and pave the way for the development of large-scale and low-cost integrated polaritonic devices operating at room temperature.

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