Proceedings of MATSUS Spring 2025 Conference (MATSUSSpring25)
DOI: https://doi.org/10.29363/nanoge.matsusspring.2025.338
Publication date: 16th December 2024
Nanostructured semiconductors dominate opto-electronics to date, mainly in the framework of quantum wells and dots grown by vacuum epitaxial methods. A next (r)evolution in this field is happening as we speak through the use of solution processable nanostructured materials. Indeed, by combining low temperature, substrate independent processing with size-tunable optical properties, such as luminescence and optical amplification (gain), these ‘nanocrystals’ are excellent building blocks to realize small footprint LEDs and lasers. In this talk, I will overview our efforts towards integrated laser sources based on colloidal nanocrystals. To do so, I will start out with discussing how optical gain, a premise to build lasers, is measured and quantified in these materials. Building on this framework, I will explain how net stimulated emission develops in and how we reached after nearly a decade of research a set of materials with excellent gain metrics on all fronts using so-called ‘bulk nanocrystals’ as a new design route. Next, I will show a few results of combining these flexible materials with integrated photonic cavities, thereby realizing ultra-small footprint lasers operating under quasi-CW pumping. Finally, I will present a route forward to transition these RGB lasers into the infrared spectrum where a select pick of ultrafast mid-infrared spectroscopy experiments gives a first flavor of the challenges , but also massive opportunities, lying ahead in the ongoing ERC project ‘NOMISS’.