Publication date: 17th February 2025
The application of hybrid organic-inorganic perovskite materials is hampered by issues related to their operational stability in response to external stimuli, such as voltage bias and light, which is associated with their mixed ionic-electronic conductivity.1–3 This can, to an extent, be overcome by incorporating tailored organic moieties within hybrid perovskite frameworks that can provide impermeability to ion migration and enable the formation of low-dimensional architectures with enhanced stability and functionality.2–3 We explore their dynamic control under operating conditions in response to voltage bias and light4–5 to enable long-term stabilization while opening perspectives toward advanced functionality beyond photovoltaics.6–7
1. S. Krause, J. V. Milić, Commun. Chem. 2023, 6, 151.
2. J. V. Milić, J. Mat. Chem. C 2021, 9, 11428.
3. J. V. Milić, Chimia 2022, 76, 784.
4. G. AlSabeh, J. V. Milić, et al. Angew. Chem. Int. Ed. 2024, accepted article
5. W. Luo, J. V. Milić, et al. 2025, manuscript under revision
6. M. Loizos, K. Rogdakis, W. Luo, P. Zimmermann, A. Hinderhofer, J. Lukić, M. Tountas,
F. Schreiber, J. V. Milić, E. Kymakis, Nanoscale Horiz. 2024, 9, 1146.
7. M. M. Ganaie, G. Bravetti, S. Sahu, M. Kumar, J. V. Milić, Mater. Adv. 2024, 5, 1880.
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