Highly reproducible large-scale perovskite solar cells fabricated via megasonic spray system
Mincheol Park a b, Woohyung Cho a, Mansoo Choi a b
a Center for Multiscale Energy Systems
b Seoul National University, Department of Mechanical and Aerospace Engineering, Seoul, Korea, Republic of
International Conference on Hybrid and Organic Photovoltaics
Proceedings of International Conference on Hybrid and Organic Photovoltaics (HOPV18)
Benidorm, Spain, 2018 May 28th - 31st
Organizers: Emilio Palomares and Rene Janssen
Poster, Mincheol Park, 229
Publication date: 21st February 2018

A simple, low-cost, versatile, and potentially scalable coating method is proposed for the fabrication of hybrid organic-inorganic perovskite solar cells. We describe a highly promising technique, the megasonic spray coating, based on an aerosol coating method with a megasonic nebulizer. Using this technique, we fabricated efficient and reproducible large-area planar perovskite solar cells. The coating is based on a mist precursor and can easily be carried out at low temperature, in a solvent free environment, and at ambient conditions. We can effectively control the volume of the CH3NH3PbI3 precursor solution and the reaction temperature, which affect the quality of the perovskite harvester layer and the performance of the perovskite solar cells. In optimized conditions, our devices reach a maximum efficiency of 16.9%, with an average efficiency of 16.4%. We also demonstrate the applicability of megasonic spray coating to the fabrication of large-area solar cells (1 cm2), with a power conversion efficiency of 14.2%.

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